| 来源类型 | Article |
| 规范类型 | 其他 |
| DOI | 10.5194/acp-16-10765-2016 |
| Multi-model evaluation of short-lived pollutant distributions over east Asia during summer 2008. | |
| Quennehen B; Raut J-C; Law K S; Daskalakis N; Ancellet G; Clerbaux C; Kim S-W; Lund M T | |
| 发表日期 | 2016 |
| 出处 | Atmospheric Chemistry and Physics 16 (17): 10765-10792 |
| 出版年 | 2016 |
| 语种 | 英语 |
| 摘要 | The ability of seven state-of-the-art chemistry–aerosol models to reproduce distributions of tropospheric ozone and its precursors, as well as aerosols over eastern Asia in summer 2008, is evaluated. The study focuses on the performance of models used to assess impacts of pollutants on climate and air quality as part of the EU ECLIPSE project. Models, run using the same ECLIPSE emissions, are compared over different spatial scales to in situ surface, vertical profiles and satellite data. Several rather clear biases are found between model results and observations, including overestimation of ozone at rural locations downwind of the main emission regions in China, as well as downwind over the Pacific. Several models produce too much ozone over polluted regions, which is then transported downwind. Analysis points to different factors related to the ability of models to simulate VOC-limited regimes over polluted regions and NOx limited regimes downwind. This may also be linked to biases compared to satellite NO2, indicating overestimation of NO2 over and to the north of the northern China Plain emission region. On the other hand, model NO2 is too low to the south and west of this region and over South Korea/Japan. Overestimation of ozone is linked to systematic underestimation of CO particularly at rural sites and downwind of the main Chinese emission regions. This is likely to be due to enhanced destruction of CO by OH. Overestimation of Asian ozone and its transport downwind implies that radiative forcing from this source may be overestimated. Model-observation discrepancies over Beijing do not appear to be due to emission controls linked to the Olympic Games in summer 2008. |
| 主题 | Air Quality & ; Greenhouse Gases (AIR) ; Mitigation of Air Pollution (MAG) |
| URL | http://pure.iiasa.ac.at/id/eprint/13811/ |
| 来源智库 | International Institute for Applied Systems Analysis (Austria) |
| 引用统计 | |
| 资源类型 | 智库出版物 |
| 条目标识符 | http://119.78.100.153/handle/2XGU8XDN/130479 |
| 推荐引用方式 GB/T 7714 | Quennehen B,Raut J-C,Law K S,et al. Multi-model evaluation of short-lived pollutant distributions over east Asia during summer 2008.. 2016. |
| 条目包含的文件 | ||||||
| 文件名称/大小 | 资源类型 | 版本类型 | 开放类型 | 使用许可 | ||
| acp-16-10765-2016.pd（5676KB） | 智库出版物 | 限制开放 | CC BY-NC-SA | 浏览 | ||
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