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来源类型Article
规范类型其他
DOI10.1038/s41561-018-0073-0
Discrepancy between simulated and observed ethane and propane levels explained by underestimated fossil fuel emissions.
Dalsøren SB; Myhre G; Hodnebrog Ø; Myhre CL; Stohl A; Pisso I; Schwietzke S; Höglund Isaksson L
发表日期2018
出处Nature Geoscience 11 (3): 178-184
出版年2018
语种英语
摘要Ethane and propane are the most abundant non-methane hydrocarbons in the atmosphere. However, their emissions, atmospheric distribution, and trends in their atmospheric concentrations are insufficiently understood. Atmospheric model simulations using standard community emission inventories do not reproduce available measurements in the Northern Hemisphere. Here, we show that observations of pre-industrial and present-day ethane and propane can be reproduced in simulations with a detailed atmospheric chemistry transport model, provided that natural geologic emissions are taken into account and anthropogenic fossil fuel emissions are assumed to be two to three times higher than is indicated in current inventories. Accounting for these enhanced ethane and propane emissions results in simulated surface ozone concentrations that are 5–13% higher than previously assumed in some polluted regions in Asia. The improved correspondence with observed ethane and propane in model simulations with greater emissions suggests that the level of fossil (geologic + fossil fuel) methane emissions in current inventories may need re-evaluation.
主题Air Quality & ; Greenhouse Gases (AIR)
URLhttp://pure.iiasa.ac.at/id/eprint/15138/
来源智库International Institute for Applied Systems Analysis (Austria)
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资源类型智库出版物
条目标识符http://119.78.100.153/handle/2XGU8XDN/131459
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Dalsøren SB,Myhre G,Hodnebrog Ø,et al. Discrepancy between simulated and observed ethane and propane levels explained by underestimated fossil fuel emissions.. 2018.
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